Glass mold created:
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Cold pressed ceramic? Looks a bit rough, but should work fine for first tests. I'm very interested in following your progress on this, hopefully with pics at each stage :) Glass molding is something I have an interest in, but I'm quite intimidated by the high temperatures needed and differences in thermal expansion coefficients of mold materials and glasses, particularly as I'm interested in eventually molding pure fused silica...
It may be possible to mold a glass "shell" of about 1mm thickness and "fill" the inside with the PU, a bit like a relegendable keycap, but joined permanently.