Hey!
What I do is I stick the synth down to a lego base plate, and build a tower around it. That will act as my mold box.
You can either put a key on the synth and sculpt on it that way, or, sculpt on the synth itself.
Once you're done sculpting,
You put the synth in the mold box, mix your silicone up, and pour it in slowly without trying to get as much air in as possible.
Wait for it to cure.
That's the mold part.
Pop the synth out when it's done curing, clean up the mold.
Lube the synth up really good with mold release. Put the base plate in the mold, pour resin into the stem hole until it is almost into the rectangular part, then you stick the stem in.
Wait for that to cure, then voila.
It will take a lot of trial and error, trust me.
I advise reading all the threads you can, and watch the livestream video of the synth.